I would like to add a lookup column in a SP list, which allows the user to select a specific library (rather than an item within that library).
Is this possible?
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You can take the following approach:
ListAddedevent. Develop your event receiver so that every time a list (or a library) is added to the web site a corresponding item is added to the Master list - for example the name of the list/library.
That way you will have a lookup (dropdown) column with the names of the lists on your site.